You can, though from personal experience it can be a bit finicky if you’re trying to emulate the better PSP version. There are some optional patches that can be applied to it to improve stability, but it still crashes on me a few times in PPSSPP.

A native PC release would have been nice to have. It’s one of the few FF games still not available on PC/Steam.

Alternatively, one could grab the Android version and try to run that on PC through the now-deprecated WSA, but the mobile port is touch input only with no controller support.